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2,4,6‐Triphenylpyridinium: A Bulky, Highly Electron‐Withdrawing Substituent That Enhances Properties of Nickel(II) Ethylene Polymerization Catalysts

Mateusz Janeta, Julius X. Heidlas, Olafs Daugulis, Maurice Brookhart

2020Angewandte Chemie International Edition24 citationsDOIOpen Access PDF

Abstract

Abstract The reactivity of Ni II and Pd II olefin polymerization catalysts can be enhanced by introduction of electron‐withdrawing substituents on the supporting ligands rendering the metal centers more electrophilic. Reported here is a comparison of ethylene polymerization activity of a classical salicyliminato nickel catalyst substituted with the powerful electron‐withdrawing 2,4,6‐triphenylpyridinium (trippy) group to the ‐CF 3 analogue. The trippy substituent is substantially more electron‐withdrawing (σ meta =0.63) than the trifluoromethyl group (σ meta =0.43) which results in a ca. 8‐fold increase in catalytic turnover frequency. An additional advantage of trippy is the high steric bulk relative to the trifluoromethyl group. This feature results in a four‐fold increase in polymer molecular weight owing to enhanced retardation of chain transfer. A significant increase in catalyst lifetime is observed as well.

Topics & Concepts

SubstituentPolar effectTrifluoromethylSteric effectsPolymerizationChemistryCatalysisPolymer chemistryEthyleneReactivity (psychology)Olefin fiberNickelPhotochemistryPolymerOrganic chemistryAlkylPathologyMedicineAlternative medicineOrganometallic Complex Synthesis and CatalysisCarbon dioxide utilization in catalysisCatalytic Alkyne Reactions
2,4,6‐Triphenylpyridinium: A Bulky, Highly Electron‐Withdrawing Substituent That Enhances Properties of Nickel(II) Ethylene Polymerization Catalysts | Litcius