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Redox‐Active Hybrid Polyoxometalate‐Stabilised Gold Nanoparticles

Carmen Martín, Katharina Kastner, Jamie M. Cameron, Elizabeth Hampson, Jesum Alves Fernandes, Emma K. Gibson, Darren A. Walsh, Víctor Sans, Graham N. Newton

2020Angewandte Chemie International Edition43 citationsDOIOpen Access PDF

Abstract

We report the design and preparation of multifunctional hybrid nanomaterials through the stabilization of gold nanoparticles with thiol-functionalised hybrid organic-inorganic polyoxometalates (POMs). The covalent attachment of the hybrid POM forms new nanocomposites that are stable at temperatures and pH values which destroy analogous electrostatically functionalised nanocomposites. Photoelectrochemical analysis revealed the unique photochemical and redox properties of these systems.

Topics & Concepts

PolyoxometalateNanomaterialsHybrid materialNanocompositeColloidal goldRedoxCovalent bondNanoparticleThiolNanotechnologyMaterials scienceChemistryCombinatorial chemistryInorganic chemistryCatalysisOrganic chemistryPolyoxometalates: Synthesis and ApplicationsNanocluster Synthesis and ApplicationsAdvanced Nanomaterials in Catalysis
Redox‐Active Hybrid Polyoxometalate‐Stabilised Gold Nanoparticles | Litcius