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Inhibition of [FeFe]-hydrogenase by formaldehyde: proposed mechanism and reactivity of FeFe alkyl complexes

Fanjun Zhang, Toby J. Woods, Lingyang Zhu, Thomas B. Rauchfuss

2021Chemical Science12 citationsDOIOpen Access PDF

Abstract

The mechanism for inhibition of [FeFe]-hydrogenases by formaldehyde is examined with model complexes.

Topics & Concepts

HydrogenaseFormaldehydeMechanism (biology)AlkylChemistryReactivity (psychology)PhotochemistryCombinatorial chemistryCatalysisOrganic chemistryPhysicsMedicineAlternative medicineQuantum mechanicsPathologyMetalloenzymes and iron-sulfur proteinsElectrocatalysts for Energy ConversionMetal-Catalyzed Oxygenation Mechanisms
Inhibition of [FeFe]-hydrogenase by formaldehyde: proposed mechanism and reactivity of FeFe alkyl complexes | Litcius