Design strategies of two-dimensional metal–organic frameworks toward efficient electrocatalysts for N<sub>2</sub> reduction: cooperativity of transition metals and organic linkers
Ran Wang, Chaozheng He, Weixing Chen, Ling Fu, Chenxu Zhao, Jinrong Huo, Chenghua Sun
Abstract
for the NRR. Therefore, our work not only demonstrates a class of promising electrocatalysts for the NRR but also provides a strategy for further predicting the catalytic activity of 2D MOFs.
Topics & Concepts
SelectivityLimitingCooperativityCatalysisTransition metalMoleculeMetalRedoxMetal-organic frameworkCombinatorial chemistryMaterials scienceChemistryNanotechnologyInorganic chemistryPhysical chemistryOrganic chemistryBiochemistryMechanical engineeringAdsorptionEngineeringAmmonia Synthesis and Nitrogen ReductionAdvanced Photocatalysis TechniquesMXene and MAX Phase Materials