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Electro-optically Modulated Nonlinear Metasurfaces

Zhengqing He, Lun Qu, Wei Wu, Jikun Liu, Chunyan Jin, Chenxiong Wang, Jingfei You, Weiye Liu, Lu Bai, Zhidong Gu, Wei Cai, Mengxin Ren, Jingjun Xu

2024Nano Letters23 citationsDOI

Abstract

Electrically reconfigurable nonlinear metasurfaces provide dynamic control over nonlinear phenomena such as second-harmonic generation (SHG), unlocking novel applications in signal processing, light switching, and sensing. Previous methods, like electric-field-induced SHG in plasmonic metasurfaces and Stark-tuned nonlinearities in quantum well metasurfaces, face limitations due to weak SHG responses from metals and mid-infrared constraints of quantum wells, respectively. Addressing the need for efficient SHG control in the visible and near-infrared ranges, we present a novel approach using the electro-optic (EO) effect to modulate SHG. By leveraging the exceptional EO and SHG properties of lithium niobate (LN), we integrate the EO effect with SHG within a metasurface framework for the first time. Our LN metasurface achieves an 11.3% modulation depth in SHG amplitude under a ±50 V alternating voltage. These results open new avenues for reconfigurable photonic applications. including tunable nonlinear light sources, quantum optics, and nonlinear information processing.

Topics & Concepts

Nonlinear opticsMaterials scienceOptoelectronicsOpticsNonlinear systemNonlinear opticalModulation (music)PhysicsNanotechnologyLaserQuantum mechanicsAcousticsMetamaterials and Metasurfaces ApplicationsPlasmonic and Surface Plasmon ResearchPhotonic Crystals and Applications