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A lysosome-targeted fluorescent probe based on a BODIPY structure for Cys/Hcy detection

Wenxuan Zhang, Binbin Wu, Manshan Liang, Mengpei Zhang, Yu‐Tao Hu, Zu‐Sheng Huang, Xiaoxia Ye, Bing Du, Yun‐Yun Quan, Yongsheng Jiang

2023Analytical Methods17 citationsDOI

Abstract

Cysteine (Cys) and homocysteine (Hcy) are important biothiols in living organisms. They play important roles in a variety of physiological and pathological processes. Therefore, it is very important to design an optical probe for the selective detection of Cys/Hcy. Herein, we report the design and synthesis of a fluorescent probe NBD-B-T based on a boron-dipyrromethene (BODIPY) structure, which showed an excellent lysosome targeting ability and an outstanding Cys/Hcy detection capacity. For NBD-B-T, the sensing group 7-nitro-2,1,3-benzoxadiazole (NBD) and the lysosomal targeting group morpholine were introduced. The results show that the NBD-B-T probe can detect Cys/Hcy with fluorescence emission turn-on performance. The low detection limits of this probe are about 76.0 nM for Hcy and 97.6 nM for Cys, respectively. The NBD-B-T probe has a low detection limit, high stability, and excellent selectivity and sensitivity. More importantly, the NBD-B-T can target lysosome, and simultaneously detect the Cys/Hcy in living cells.

Topics & Concepts

BODIPYChemistryFluorescenceLysosomeCysteineDetection limitBiophysicsBiochemistryBiologyEnzymeChromatographyPhysicsQuantum mechanicsSulfur Compounds in BiologyMolecular Sensors and Ion DetectionNanoplatforms for cancer theranostics
A lysosome-targeted fluorescent probe based on a BODIPY structure for Cys/Hcy detection | Litcius