Two-dimensional materials as a stabilized interphase for the solid-state electrolyte Li<sub>10</sub>GeP<sub>2</sub>S<sub>12</sub> in lithium metal batteries
Jiachen Ma, Ruge Quhe, Zheyu Zhang, Chen Yang, Xiuying Zhang, Jingzhen Li, Lin Xu, Jie Yang, Bowen Shi, Shiqi Liu, Linqiang Xu, Xiaotian Sun, Jing Lü
Abstract
An efficient screening procedure for two-dimensional (2D) solid-electrolyte interphases (SEIs) is designed. In the concrete case, the two selected 2D SEIs (<italic>h</italic>-BN and <italic>α</italic>-BNyne) do stabilize the interface between the solid-state electrolyte Li<sub>10</sub>GeP<sub>2</sub>S<sub>12</sub> and the lithium metal anode, blocking the electron transfer and maintaining the Li-ion flow.
Topics & Concepts
ElectrolyteLithium (medication)AnodeLithium metalInterphaseSolid-stateMaterials scienceFast ion conductorMetalInorganic chemistryChemistryAnalytical Chemistry (journal)ElectrodePhysical chemistryMetallurgyGeneticsChromatographyMedicineEndocrinologyBiologyAdvanced Battery Materials and TechnologiesAdvancements in Battery MaterialsInorganic Chemistry and Materials