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TEMPO Radical-Functionalized Supramolecular Coordination Complexes with Controllable Spin–Spin Interactions

Wei‐Ling Jiang, Zhiyong Peng, Bin Huang, Xiao‐Li Zhao, Di Sun, Xueliang Shi, Hai‐Bo Yang

2020Journal of the American Chemical Society42 citationsDOI

Abstract

via the crystal-to-amorphous transformation induced by mechanical grinding and solvent vapor stimuli was also successfully realized. The unique and controllable inter- and intramolecular spin-spin interactions in this work reveal new insights for the understanding and manipulation of spin-spin interactions and may open up a new way to develop organic spin materials in the future.

Topics & Concepts

Intramolecular forceChemistrySupramolecular chemistryIntermolecular forceElectron paramagnetic resonanceCrystallographyZero field splittingCounterionSpin (aerodynamics)Spin statesChemical physicsPulsed EPRSpin polarizationCrystal structureStereochemistrySpin echoMoleculeNuclear magnetic resonanceElectronIonPhysicsInorganic chemistryRadiologyThermodynamicsMedicineQuantum mechanicsOrganic chemistryMagnetic resonance imagingMagnetism in coordination complexesMetal-Organic Frameworks: Synthesis and ApplicationsSupramolecular Chemistry and Complexes
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