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Asymmetric chlorination of A<sub>2</sub>–A<sub>1</sub>–D–A<sub>1</sub>–A<sub>2</sub> type non-fullerene acceptors for high-voltage organic photovoltaics

Peiqing Cong, Xianda Li, Ailing Tang, Jiang Wu, Jianhua Chen, Lie Chen, Erjun Zhou

2022Chemical Communications24 citationsDOI

Abstract

We synthesized the first asymmetric A 2 –A 1 –D–A 1 –A 2 type small molecule nonfullerene acceptor, HCl-BTA3 , by chlorination on one side of the A 1 unit, yielding a high open-circuit voltage of 1.20 V and a satisfactory power conversion efficiency of 11.2%.

Topics & Concepts

AcceptorFullereneEnergy conversion efficiencyOrganic solar cellCarboxylateOpen-circuit voltageMoleculeChemistryDipolePhotovoltaicsPolymerVoltagePhotovoltaic systemMaterials scienceOrganic chemistryOptoelectronicsCondensed matter physicsBiologyQuantum mechanicsPhysicsEcologyOrganic Electronics and PhotovoltaicsConducting polymers and applicationsAdvanced battery technologies research
Asymmetric chlorination of A<sub>2</sub>–A<sub>1</sub>–D–A<sub>1</sub>–A<sub>2</sub> type non-fullerene acceptors for high-voltage organic photovoltaics | Litcius