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Discovery of two new isomers of cyanoacenaphthylene (C <sub>12</sub> H <sub>7</sub> CN) in the Taurus molecular cloud 1 with the QUIJOTE line survey

J. Cernicharo, B. Tercero, N. Marcelino, J. A. López-Pérez, J. D. Gallego, F. Tercero, G. Esplugues, C. Cabezas, M. Agúndez, C. Limeres, Amanda L. Steber, Dolores Pérez, Cristóbal Pérez, Alberto Lesarri, P. de Vicente

2025Astronomy and Astrophysics8 citationsDOIOpen Access PDF

Abstract

We report the discovery of the 3- and 4-cyano isomers of acenaphthylene (C 12 H 8 ) using the QUIJOTE line survey of the Taurus molecular cloud 1 (TMC-1). The frequency range of the line survey in the Q band (31.2–50.3 GHz) was complemented with data from a new receiver installed at the Yebes 40m radio telescope that covers the K and K a bands (18–32 GHz). The identification of 3-cyanoacenaphthylene was based on the detection of 135 individual lines that correspond to 194 rotational transitions. For 4-cyanoacenaphthylene, the lines are slightly weaker, but we identified 37 individual lines that correspond to 66 rotational transitions. As a first step for the identification, we compared the derived rotational constants with their expected theoretical values and obtained a match better than 0.2%. Finally, the new isomers were synthesized in our chemical laboratory and observed in our microwave spectroscopic facilities. The derived laboratory constants match those derived from TMC-1 data perfectly, which confirms our identifications. Lines in the K − K a band from the previously detected isomers 1- and 5-cyanoacenaphthylene are also reported. The derived column density for 3-cyanoacenaphthylene is (7.0 ± 0.7) × 10 11 cm −2 , and for the 4-cyano isomer, we derive a column density of (5.0 ± 0.6) × 10 11 cm −2 . The four possible isomers of cyanoacenaphthylene are finally found in TMC-1. Despite their high relative energies, they exhibit similar abundances (within a factor of ∼2).

Topics & Concepts

PhysicsAstrophysicsMolecular cloudLine (geometry)MicrowaveCosmic microwave backgroundSpectral lineEmission spectrumTelescopeRotational spectroscopyRange (aeronautics)AstrochemistryAstronomyRotational transitionMoleculeGreen Bank TelescopeAcenaphthyleneRadio telescopeAnalytical Chemistry (journal)Optical depthProtostarAstrophysics and Star Formation StudiesMolecular Spectroscopy and StructureAstro and Planetary Science
Discovery of two new isomers of cyanoacenaphthylene (C <sub>12</sub> H <sub>7</sub> CN) in the Taurus molecular cloud 1 with the QUIJOTE line survey | Litcius