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Anthracene‐Fused Oligo‐BODIPYs: A New Class of π‐Extended NIR‐Absorbing Materials

Jorge Labella, Gonzalo Durán‐Sampedro, Swathi Krishna, M. Victoria Martínez‐Díaz, Dirk M. Guldi, Tomás Torres⊗

2022Angewandte Chemie International Edition35 citationsDOIOpen Access PDF

Abstract

-catalyzed cyclization a series of fully π-conjugated anthracene-fused oligo-BODIPYs. Their structural and optoelectronic properties were studied by several techniques, ranging from X-ray, UV/Vis, and cyclic voltammetry to transient absorption spectroscopy. As a complement, their electronic structures were explored by means of Density Functional Theory (DFT) calculations. Depending on the size and shape of the π-conjugated skeleton, unique features-such as face-to-face supramolecular organization, NIR absorption and fluorescence as well as strong electron accepting character-were noted. All in all, the aforementioned features render them valuable for technological applications.

Topics & Concepts

AnthraceneConjugated systemCyclic voltammetrySupramolecular chemistryAbsorption (acoustics)Absorption spectroscopyFluorescencePhotochemistryDensity functional theoryMaterials scienceSpectroscopyChemistryMoleculePolymerOrganic chemistryElectrochemistryComputational chemistryOpticsElectrodePhysical chemistryPhysicsComposite materialQuantum mechanicsLuminescence and Fluorescent MaterialsPorphyrin and Phthalocyanine ChemistryOrganic Light-Emitting Diodes Research