Litcius/Paper detail

Laser-based angle-resolved photoemission spectroscopy with micrometer spatial resolution and detection of three-dimensional spin vector

Takuma Iwata, T. Kousa, Yasushiro Nishioka, Kenji Ohwada, Kazuki Sumida, E. Annese, Masaaki Kakoki, Kenta Kuroda, Hideaki Iwasawa, Masashi Arita, Shiv Kumar, A. Kimura, K. Miyamoto, Taichi Okuda

2024Scientific Reports15 citationsDOIOpen Access PDF

Abstract

We have developed a state-of-the-art apparatus for laser-based spin- and angle-resolved photoemission spectroscopy with micrometer spatial resolution (µ-SARPES). This equipment is realized by the combination of a high-resolution photoelectron spectrometer, a 6 eV laser with high photon flux that is focused down to a few micrometers, a high-precision sample stage control system, and a double very-low-energy-electron-diffraction spin detector. The setup achieves an energy resolution of 1.5 (5.5) meV without (with) the spin detection mode, compatible with a spatial resolution better than 10 µm. This enables us to probe both spatially-resolved electronic structures and vector information of spin polarization in three dimensions. The performance of µ-SARPES apparatus is demonstrated by presenting ARPES and SARPES results from topological insulators and Au photolithography patterns on a Si (001) substrate.

Topics & Concepts

Angle-resolved photoemission spectroscopyPhotoemission spectroscopyLaserMaterials scienceSpectroscopyInverse photoemission spectroscopyResolution (logic)OpticsDetectorX-ray photoelectron spectroscopyImage resolutionSpectrometerOptoelectronicsPhysicsElectronic structureNuclear magnetic resonanceCondensed matter physicsComputer scienceQuantum mechanicsArtificial intelligenceElectronic and Structural Properties of OxidesTopological Materials and PhenomenaPhysics of Superconductivity and Magnetism