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A mononuclear divalent ytterbium hydrido complex supported by a super-bulky scorpionate ligand

Xianghui Shi, Peng Deng, Thayalan Rajeshkumar, Lanxiao Zhao, Laurent Maron, Jianhua Cheng

2021Chemical Communications16 citationsDOI

Abstract

= hydrotris(3-adamantyl-5-isopropyl-pyrazolyl)borate) (2) bearing a terminal hydrido ligand was obtained by hydrogenolysis of the benzyl precursor in hexane. Complex 2 exhibited two different reaction patterns towards allenes: Yb-H addition with cyclohexylallene and deprotonation of 1,1-dimethylallene.

Topics & Concepts

YtterbiumDivalentChemistryHydrogenolysisLigand (biochemistry)HydrideIsopropylHexaneMedicinal chemistryInorganic chemistryOrganic chemistryCatalysisMetalReceptorMaterials scienceDopingBiochemistryOptoelectronicsOrganometallic Complex Synthesis and CatalysisCarbon dioxide utilization in catalysisInorganic Chemistry and Materials