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Tuning the Fluorescence and the Intramolecular Charge Transfer of Phenothiazine Dipolar and Quadrupolar Derivatives by Oxygen Functionalization

Yogajivan Rout, Chiara Montanari, Erika Pasciucco, Rajneesh Misra, Benedetta Carlotti

2021Journal of the American Chemical Society134 citationsDOIOpen Access PDF

Abstract

, with the fluorescence being thus significantly quenched. These results prove oxygen functionalization as a new effective synthetic strategy to tailor the photophysics of phenothiazine-based organic materials for different optoelectronic applications. While oxygen-functionalized compounds are highly fluorescent and promising active materials for current-to-light conversion in organic light-emitting diode devices, oxygen-free systems show very efficient photoinduced ICT and may be employed for light-to-current conversion in organic photovoltaics.

Topics & Concepts

ChemistryPhotochemistryPhenothiazineIntramolecular forceChromophoreUltrafast laser spectroscopySinglet oxygenFluorescenceAbsorption (acoustics)Electron transferSurface modificationOxygenPhysical chemistryStereochemistryOrganic chemistryMaterials scienceSpectroscopyPharmacologyQuantum mechanicsComposite materialPhysicsMedicineOrganic Light-Emitting Diodes ResearchPerovskite Materials and ApplicationsNonlinear Optical Materials Research
Tuning the Fluorescence and the Intramolecular Charge Transfer of Phenothiazine Dipolar and Quadrupolar Derivatives by Oxygen Functionalization | Litcius