Litcius/Paper detail

Insertion of Diazo Esters into C–F Bonds toward Diastereoselective One-Carbon Elongation of Benzylic Fluorides: Unprecedented BF<sub>3</sub> Catalysis with C–F Bond Cleavage and Re-formation

Fei Wang, Yoshihiro Nishimoto, Makoto Yasuda

2021Journal of the American Chemical Society52 citationsDOI

Abstract

Selective transformation of C–F bonds remains a significant goal in organic chemistry, but C–F insertion of a one-carbon-atom unit has never been established. Herein we report the BF3-catalyzed formal insertion of diazo esters as one-carbon-atom sources into C–F bonds to accomplish one-carbon elongation of benzylic fluorides. A DFT calculation study revealed that the BF3 catalyst could contribute to both C–F bond cleavage and re-formation. This elongation provided α-fluoro-α,β-diaryl esters with a high level of diastereoselectivity. Various benzylic fluorides and diazo esters were applicable. The synthetic utility of this method was demonstrated by the synthesis of a fluoro analogue of a compound that is used as a transient receptor and potential canonical channel inhibitor.

Topics & Concepts

ChemistryDiazoCatalysisElongationBond cleavageCarbon fibersCarbon atomCleavage (geology)StereochemistryMedicinal chemistryOrganic chemistryRing (chemistry)Composite numberEngineeringMetallurgyFracture (geology)Composite materialGeotechnical engineeringMaterials scienceUltimate tensile strengthFluorine in Organic ChemistryInorganic Fluorides and Related CompoundsCyclopropane Reaction Mechanisms
Insertion of Diazo Esters into C–F Bonds toward Diastereoselective One-Carbon Elongation of Benzylic Fluorides: Unprecedented BF<sub>3</sub> Catalysis with C–F Bond Cleavage and Re-formation | Litcius