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Machine Learning‐Assisted Microfluidic Synthesis of Perovskite Quantum Dots

Gaoyu Chen, Xia Zhu, Chenyu Xing, Yongkai Wang, Xiangxing Xu, Jianchun Bao, Jinghan Huang, Yurong Zhao, Xuan Wang, Xuan Wang, Xiuqing Zhou, Xiuli Du, Xun Wang, Xun Wang

2022Advanced Photonics Research31 citationsDOIOpen Access PDF

Abstract

The quality and property control of nanomaterials are center themes to guarantee and promote their applications. Different synthesis methods and reaction parameters are control factors for their properties. However, the vast combination number of the factors with multilevels leads to the obstacle that trying all‐through the data space is nearly impossible. Herein, the combination of microfluidic synthesis method with machine learning (ML) models to address this challenge in case of perovskite quantum dots (PQDs) with tunable photoluminescence (PL) is reported. The ML‐assisted synthesis not only helps to elucidate the nucleation growth‐ripening mechanisms, but also successfully guides to synthesize PQDs with precise wavelength and full width of half maximum (FWHM) of the PL by optimizable conditions to match the time‐saving, energy‐saving, and minimal environmental pressure goals.

Topics & Concepts

Perovskite (structure)Quantum dotNucleationFull width at half maximumPhotoluminescenceMaterials scienceNanomaterialsMicrofluidicsNanotechnologyEnergy (signal processing)Quality (philosophy)Computer scienceOptoelectronicsChemical engineeringPhysicsEngineeringQuantum mechanicsThermodynamicsPerovskite Materials and ApplicationsQuantum Dots Synthesis And PropertiesAdvanced Photocatalysis Techniques