Anomalous Hall conductivity control in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi>Mn</mml:mi></mml:mrow><mml:mn>3</mml:mn></mml:msub><mml:mi>NiN</mml:mi></mml:math> antiperovskite by epitaxial strain along the kagome plane

Abstract

Antiferromagnetic manganese-based nitride antiperovskites, such as ${\mathrm{Mn}}_{3}\mathrm{NiN}$, hold a triangular frustrated magnetic ordering, thanks to their kagome lattice formed by the Mn atoms along the (111) plane. As such, the magnetic frustration imposes a nontrivial interplay between the symmetric and asymmetric magnetic interactions, which can only reach equilibrium in a noncollinear magnetic configuration. Consequently, the associated electronic interactions and their possible tuning by external constraints, such as applied epitaxial strain, play a crucial role in defining the microscopic and macroscopic properties of such topological condensed matter systems. In this paper, we explored and explained the effect of the epitaxial strain imposed within the (111) plane, in which the magnetic and crystallographic symmetry operations are kept fixed, and only the magnitude of the ionic and electronic interactions are tuned. We found a tangible enhancement in the anomalous Hall conductivity along the (111) plane (${\ensuremath{\sigma}}_{111}^{\mathrm{AHE}}$) for compression values, whereas, for tension, the AHC is dramatically reduced. As such, the ${\ensuremath{\sigma}}_{111}^{\mathrm{AHE}}$ component fetches a maximum increase of 26%, with respect to the unstrained structure, for a compression value close to $\ensuremath{-}1.5%$. Our findings indicate a distinct correlation between the anomalous Hall conductivity and the Berry curvature along the (111) plane as a function of the strain. Here, the nondivergent Berry curvature acts as the source and the strain as the control mechanism of this anomalous transport phenomenon.

Topics & Concepts