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Magnetic and electronic properties unveil polaron formation in Eu$$_5$$In$$_2$$Sb$$_6$$

M. Victoria Ale Crivillero, Sahana Rößler, S. Granovsky, M. Doerr, Matthew S. Cook, P. F. S. Rosa, Jens Müller, S. Wirth

2023Scientific Reports18 citationsDOIOpen Access PDF

Abstract

The intermetallic compound Eu[Formula: see text]In[Formula: see text]Sb[Formula: see text], an antiferromagnetic material with nonsymmorphic crystalline structure, is investigated by magnetic, electronic transport and specific heat measurements. Being a Zintl phase, insulating behavior is expected. Our thermodynamic and magnetotransport measurements along different crystallographic directions strongly indicate polaron formation well above the magnetic ordering temperatures. Pronounced anisotropies of the magnetic and transport properties even above the magnetic ordering temperature are observed despite the Eu[Formula: see text] configuration which testify to complex and competing magnetic interactions between these ions and give rise to intricate phase diagrams discussed in detail. Our results provide a comprehensive framework for further detailed study of this multifaceted compound with possible nontrivial topology.

Topics & Concepts

AntiferromagnetismIntermetallicPolaronCondensed matter physicsAnisotropyMaterials scienceIonPhase (matter)Chemical physicsChemistryPhysicsAlloyComposite materialElectronQuantum mechanicsOrganic chemistryPhysics of Superconductivity and MagnetismMagnetic and transport properties of perovskites and related materialsRare-earth and actinide compounds
Magnetic and electronic properties unveil polaron formation in Eu$_5$In$_2$Sb$_6$ | Litcius