Litcius/Paper detail

A General Strategy to Glassy M‐Te (M = Ru, Rh, Ir) Porous Nanorods for Efficient Electrochemical N<sub>2</sub> Fixation

Juan Wang, Bolong Huang, Yujin Ji, Mingzi Sun, Tong Wu, Rongguan Yin, Xing Zhu, Youyong Li, Qi Shao, Xiaoqing Huang

2020Advanced Materials149 citationsDOIOpen Access PDF

Abstract

Abstract Electrochemical conversion of nitrogen (N 2 ) into value‐added ammonia (NH 3 ) is highly desirable yet formidably challenging due to the extreme inertness of the N 2 molecule, which makes the development of a robust electrocatalyst prerequisite. Herein, a new class of bullet‐like M‐Te (M = Ru, Rh, Ir) glassy porous nanorods (PNRs) is reported as excellent electrocatalysts for N 2 reduction reaction (NRR). The optimized IrTe 4 PNRs present superior activity with the highest NH 3 yield rate (51.1 µg h −1 mg −1 cat. ) and Faraday efficiency (15.3%), as well as long‐term stability of up to 20 consecutive cycles, making them among the most active NRR electrocatalysts reported to date. Both the N 2 temperature‐programmed desorption and valence band X‐ray photoelectron spectroscopy data show that the strong chemical adsorption of N 2 is the key for enhancing the NRR and suppressing the hydrogen evolution reaction of IrTe 4 PNRs. Density functional theory calculations comprehensively identify that the superior adsorption strength of IrTe 4 adsorptions originates from the synergistic collaboration between electron‐rich Ir and the highly electroactive surrounding Te atoms. The optimal adsorption of both N 2 and H 2 O in alkaline media guarantees the superior consecutive NRR process. This work opens a new avenue for designing high‐performance NRR electrocatalysts based on glassy materials.

Topics & Concepts

Materials scienceNanorodElectrochemistryElectrocatalystX-ray photoelectron spectroscopyDesorptionAdsorptionReversible hydrogen electrodeChemical engineeringNanotechnologyInorganic chemistryPhysical chemistryChemistryElectrodeWorking electrodeEngineeringAmmonia Synthesis and Nitrogen ReductionAdvanced Photocatalysis TechniquesCatalytic Processes in Materials Science