Litcius/Paper detail

Dual role of benzophenone enables a fast and scalable C-4 selective alkylation of pyridines in flow

Jesús Sanjosé‐Orduna, Rodrigo C. Silva, Fabian Raymenants, Bente Reus, Jannik Thaens, Kléber T. de Oliveira, Timothy Noël

2022Chemical Science20 citationsDOIOpen Access PDF

Abstract

a HAT mechanism, and by acting as a benign, terminal oxidant. The key role of benzophenone in the operative reaction mechanism has also been revealed through a combination of experimental and computational studies.

Topics & Concepts

BenzophenoneAlkylationChemistryRadicalRegioselectivityCombinatorial chemistryAlkylPyridinePhotochemistryOrganic chemistryCatalysisInnovative Microfluidic and Catalytic Techniques InnovationRadical Photochemical ReactionsCatalytic C–H Functionalization Methods