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Si-Integrated BaTiO<sub>3</sub> for Electro-Optic Applications: Crystalline and Polarization Orientation Control

Marc Reynaud, Huaixun Huyan, Chaojie Du, Wente Li, Agham Posadas, Xiaoqing Pan, Alexander A. Demkov

2023ACS Applied Electronic Materials10 citationsDOI

Abstract

Recent research has demonstrated that BaTiO 3 epitaxially grown on Si is capable of a large electro-optical response via the Pockels effect crucial for fabricating efficient phase modulators in integrated silicon photonics. However, the typical crystallographic orientation evolution of epitaxial BaTiO 3 on SrTiO 3 -buffered Si yields a dead layer (a region of the film with a low electro-optic response) for most device geometries. We report on a Si-on-insulator-integrated film stack incorporating a MgO buffer layer that effectively alleviates this problem. The film quality is confirmed with crystallographic characterization; electro-optic measurements yield an effective Pockels coefficient of 119 pm/V for a 100 nm thick film.

Topics & Concepts

Pockels effectMaterials scienceEpitaxyOptoelectronicsPolarization (electrochemistry)Insulator (electricity)PhotonicsLayer (electronics)Silicon on insulatorSiliconOpticsLaserNanotechnologyChemistryPhysicsPhysical chemistryPhotonic and Optical DevicesPhotorefractive and Nonlinear OpticsSemiconductor materials and devices
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