Litcius/Paper detail

Characterization of temperature distributions in a swirled oxy-fuel coal combustor using tomographic absorption spectroscopy with fluctuation modelling

Johannes Emmert, Henrik Schneider, Christian Meißner, Evaggelos Sidiropoulos, Jonas I. Hölzer, Thomas Seeger, Benjamin Böhm, Andreas Dreizler, Steven Wagner

2021Applications in Energy and Combustion Science19 citationsDOIOpen Access PDF

Abstract

Oxy-fuel combustion promises efficient and inexpensive carbon dioxide sequestration and is therefore subject to active experimental research. However, the transfer of mature, non-intrusive diagnostic methods for temperature measurement like Coherent Anti-Stokes Raman Spectroscopy (CARS) from air-fed to oxy-fuel systems is challenging due to the deficiency in diatomic species suitable for thermometry. Although not limited to oxy-fuel atmospheres, we demonstrate the application of linear hyperspectral absorption tomography on water vapor in a swirled oxy-fuel coal combustor as a complementary diagnostic method, supplementing reference and validation data sets. Due to the burner design an axisymmetric reconstruction of the time-averaged temperature field is conducted. To compensate the temperature bias expected when evaluating time-averaged spectroscopic data we incorporate turbulent temperature fluctuations into our spectroscopic model, providing a fluctuation measure in addition to mean temperatures. The results quantitatively agree with vibrational O2-CARS measurements and qualitatively recreate spatial structures known from particle image velocimetry (PIV) flow fields.

Topics & Concepts

CombustorCombustionRaman spectroscopyAbsorption (acoustics)Temperature measurementMaterials scienceComputational physicsWater vaporTurbulenceAnalytical Chemistry (journal)Environmental scienceMechanicsNuclear engineeringMeteorologyOpticsChemistryThermodynamicsPhysicsEngineeringChromatographyOrganic chemistryCombustion and flame dynamicsAtmospheric and Environmental Gas DynamicsSpectroscopy and Laser Applications