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Rhodium(<scp>iii</scp>)-catalyzed C–H/C–F activation sequence: expedient and divergent synthesis of 2-benzylated indoles and 2,2′-bis(indolyl)methanes

Bing Shu, Shaoyong Chen, Nan-Xiang Deng, Tao Zheng, Hui Xie, Xiaoling Xie, Jia‐Qiang Wu, Hua Cao, Shang‐Shi Zhang

2021Organic Chemistry Frontiers25 citationsDOI

Abstract

A novel method for the construction of fluorinated 2-benzylated indoles and 2,2’-bis(indolyl)methanes was developed <italic>via</italic> Rh(<sc>iii</sc>)-catalyzed C–H/C–F activation of arenes with employing 3,3-difluoro-2-exo-methylidene indolines as cross-coupling partner.

Topics & Concepts

ChemistryRhodiumCatalysisSequence (biology)Medicinal chemistryStereochemistryOrganic chemistryBiochemistryFluorine in Organic ChemistryCatalytic C–H Functionalization MethodsSynthesis and Catalytic Reactions
Rhodium(<scp>iii</scp>)-catalyzed C–H/C–F activation sequence: expedient and divergent synthesis of 2-benzylated indoles and 2,2′-bis(indolyl)methanes | Litcius