Electrostatic [FeFe]-hydrogenase–carbon nitride assemblies for efficient solar hydrogen production
Yongpeng Liu, Carolina Pulignani, Sophie Webb, Samuel J. Cobb, Santiago Rodríguez‐Jiménez, Dong-Seok Kim, Ross D. Milton, Erwin Reisner
Abstract
(4 h) and a turnover number (TON) of 198 125 (24 h). Interfacial characterizations, including quartz crystal microbalance (QCM), photoelectrochemical impedance spectroscopy (PEIS), intensity-modulated photovoltage spectroscopy (IMVS), and transient photocurrent spectroscopy (TPC) have been conducted on the semi-artificial carbon nitride-enzyme system to provide a comprehensive understanding for the future development of photocatalytic hybrid assemblies.
Topics & Concepts
HydrogenaseCarbon nitrideHydrogen productionMaterials scienceHydrogenNanotechnologyCarbon fibersNitrideWater splittingPhotochemistryChemical engineeringChemistryPhotocatalysisCatalysisOrganic chemistryEngineeringComposite materialComposite numberLayer (electronics)Electrocatalysts for Energy ConversionMetalloenzymes and iron-sulfur proteinsAdvanced Photocatalysis Techniques