Surface hydroxyl group dominating aerobic oxidation of methane below room temperature
Baiyang Yu, Lu Cheng, Jiaju Wu, Bing Yang, Hong Li, Jing Xu, Ying Zhang, Chengsi Pan, Xiaoming Cao, Yongfa Zhu, Yang Lou
Abstract
Titanium silicate-supported single Pd atoms coated with ultrathin N-doped carbon (Pd 1 /TS-1@CN) as an efficient and stable catalyst enabling direct oxidation of methane to value-added products with 100% selectivity by O 2 and H 2 at 15 °C.
Topics & Concepts
MethaneAnaerobic oxidation of methaneGroup (periodic table)ChemistryMaterials sciencePhotochemistryOrganic chemistryAtmospheric and Environmental Gas DynamicsCatalysis and Oxidation Reactions