Litcius/Paper detail

Functional Group Evaluation Kit for Digitalization of Information on the Functional Group Compatibility and Chemoselectivity of Organic Reactions

Natsuki Saito, Anna Nawachi, Yuta Kondo, Jeesoo Choi, Hiroyuki Morimoto, Takashi Ohshima

2023Bulletin of the Chemical Society of Japan31 citationsDOI

Abstract

Abstract Digitalization of information on organic reactions is essential for developing next-generation organic syntheses with artificial intelligence and machine-learning (ML) methods. In this regard, reliable information on functional group compatibility and chemoselectivity is critical for understanding the applicability of the reactions. Herein, we report the digitalization of organic reactions using a functional group evaluation (FGE) kit that allows for accurate and rapid assessment of information on the functional group compatibility and chemoselectivity of given organic reactions. Our 26 FGE compounds were used to evaluate 4 types of organic reactions (i.e., cross-coupling, proline-catalyzed aldol, condensation, and ketimine synthesis reactions). As a result, we obtained valuable information for developing a new model of retrosynthetic analysis tools and a deeper understanding of these reactions.

Topics & Concepts

ChemoselectivityChemistryFunctional groupCompatibility (geochemistry)Retrosynthetic analysisOrganic reactionCombinatorial chemistryOrganic chemistryCatalysisTotal synthesisChemical engineeringEngineeringPolymerAsymmetric Hydrogenation and CatalysisMachine Learning in Materials ScienceCatalytic C–H Functionalization Methods