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Hyperuniform Structures Formed by Shearing Colloidal Suspensions

Sam Wilken, Rodrigo Guerra, David J. Pine, P. M. Chaikin

2020Physical Review Letters56 citationsDOIOpen Access PDF

Abstract

In periodically sheared suspensions there is a dynamical phase transition, characterized by a critical strain amplitude γ_{c}, between an absorbing state where particle trajectories are reversible and an active state where trajectories are chaotic and diffusive. Repulsive nonhydrodynamic interactions between "colliding" particles' surfaces have been proposed as a source of this broken time reversal symmetry. A simple toy model called random organization qualitatively reproduces the dynamical features of this transition. Random organization and other absorbing state models exhibit hyperuniformity, a strong suppression of density fluctuations on long length scales quantified by a structure factor S(q→0)∼q^{α} with α>0, at criticality. Here we show experimentally that the particles in periodically sheared suspensions organize into structures with anisotropic short-range order but isotropic, long-range hyperuniform order when oscillatory shear amplitudes approach γ_{c}.

Topics & Concepts

Shearing (physics)IsotropyAmplitudePhysicsAnisotropyPhase transitionCondensed matter physicsQuantum mechanicsThermodynamicsMaterial Dynamics and PropertiesPickering emulsions and particle stabilizationLiquid Crystal Research Advancements