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Enhanced photoelectrochemical water splitting performance of α-Fe<sub>2</sub>O<sub>3</sub> photoanodes through Co-modification with Co single atoms and g-C<sub>3</sub>N<sub>4</sub>

Juan Wu, Xiaodi Du, Mingjie Li, Hongyu Chen, Bin Hu, Hongwei Ding, Nannan Wang, Lin Jin, Weisheng Liu

2024Chemical Science11 citationsDOIOpen Access PDF

Abstract

served as a suitable carrier for single atoms, which effectively anchored CoSAs through N/C coordination. The highly dispersed CoSAs provided abundant active sites, which further promoted surface holes extraction and oxidation kinetics, resulting in higher PEC performance and photostability. This study indicates the benefits of these collaborative strategies and provides more efficient designs for solar energy conversion in PEC systems.

Topics & Concepts

Water splittingPhotoelectrochemistryMaterials scienceCrystallographyChemistryCatalysisPhotocatalysisElectrochemistryPhysical chemistryElectrodeBiochemistryIron oxide chemistry and applicationsAdvanced Photocatalysis TechniquesAdvanced oxidation water treatment