Absence of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>E</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn><mml:mi>g</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math> Nematic Instability and Dominant <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>A</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mi>g</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math> Response in the Kagome Metal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>CsV</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi>Sb</mml:mi></mml:mrow><mml:mrow><mml:mn>5</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>
Zhaoyu Liu, Yue Shi, Qianni Jiang, Elliott Rosenberg, Jonathan M. DeStefano, Jinjin Liu, Chaowei Hu, Yuzhou Zhao, Zhiwei Wang, Yugui Yao, David Graf, Pengcheng Dai, Jihui Yang, Xiaodong Xu, Jiun‐Haw Chu
Abstract
Ever since the discovery of the charge density wave (CDW) transition in the kagome metal <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msub><a:mrow><a:mi>CsV</a:mi></a:mrow><a:mrow><a:mn>3</a:mn></a:mrow></a:msub></a:mrow><a:mrow><a:msub><a:mrow><a:mi>Sb</a:mi></a:mrow><a:mrow><a:mn>5</a:mn></a:mrow></a:msub></a:mrow></a:math>, the nature of its symmetry breaking has been under intense debate. While evidence suggests that the rotational symmetry is already broken at the CDW transition temperature (<c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:msub><c:mi>T</c:mi><c:mrow><c:mi>CDW</c:mi></c:mrow></c:msub></c:math>), an additional electronic nematic instability well below <e:math xmlns:e="http://www.w3.org/1998/Math/MathML" display="inline"><e:msub><e:mi>T</e:mi><e:mrow><e:mi>CDW</e:mi></e:mrow></e:msub></e:math> has been reported based on the diverging elastoresistivity coefficient in the anisotropic channel (<g:math xmlns:g="http://www.w3.org/1998/Math/MathML" display="inline"><g:msub><g:mi>m</g:mi><g:msub><g:mi>E</g:mi><g:mrow><g:mn>2</g:mn><g:mi>g</g:mi></g:mrow></g:msub></g:msub></g:math>). Verifying the existence of a nematic transition below <i:math xmlns:i="http://www.w3.org/1998/Math/MathML" display="inline"><i:msub><i:mi>T</i:mi><i:mrow><i:mi>CDW</i:mi></i:mrow></i:msub></i:math> is not only critical for establishing the correct description of the CDW order parameter, but also important for understanding low-temperature superconductivity. Here, we report elastoresistivity measurements of <k:math xmlns:k="http://www.w3.org/1998/Math/MathML" display="inline"><k:mrow><k:msub><k:mrow><k:mi>CsV</k:mi></k:mrow><k:mrow><k:mn>3</k:mn></k:mrow></k:msub></k:mrow><k:mrow><k:msub><k:mrow><k:mi>Sb</k:mi></k:mrow><k:mrow><k:mn>5</k:mn></k:mrow></k:msub></k:mrow></k:math> using three different techniques probing both isotropic and anisotropic symmetry channels. Contrary to previous reports, we find the anisotropic elastoresistivity coefficient <m:math xmlns:m="http://www.w3.org/1998/Math/MathML" display="inline"><m:msub><m:mi>m</m:mi><m:msub><m:mi>E</m:mi><m:mrow><m:mn>2</m:mn><m:mi>g</m:mi></m:mrow></m:msub></m:msub></m:math> is temperature independent, except for a step jump at <o:math xmlns:o="http://www.w3.org/1998/Math/MathML" display="inline"><o:msub><o:mi>T</o:mi><o:mrow><o:mi>CDW</o:mi></o:mrow></o:msub></o:math>. The absence of nematic fluctuations is further substantiated by measurements of the elastocaloric effect, which show no enhancement associated with nematic susceptibility. On the other hand, the symmetric elastoresistivity coefficient <q:math xmlns:q="http://www.w3.org/1998/Math/MathML" display="inline"><q:msub><q:mi>m</q:mi><q:msub><q:mi>A</q:mi><q:mrow><q:mn>1</q:mn><q:mi>g</q:mi></q:mrow></q:msub></q:msub></q:math> increases below <s:math xmlns:s="http://www.w3.org/1998/Math/MathML" display="inline"><s:msub><s:mi>T</s:mi><s:mrow><s:mi>CDW</s:mi></s:mrow></s:msub></s:math>, reaching a peak value of 90 at <u:math xmlns:u="http://www.w3.org/1998/Math/MathML" display="inline"><u:msup><u:mi>T</u:mi><u:mo>*</u:mo></u:msup><u:mo>=</u:mo><u:mn>20</u:mn><u:mtext> </u:mtext><u:mtext> </u:mtext><u:mi mathvariant="normal">K</u:mi></u:math>. Our results strongly indicate that the phase transition at <x:math xmlns:x="http://www.w3.org/1998/Math/MathML" display="inline"><x:msup><x:mi>T</x:mi><x:mo>*</x:mo></x:msup></x:math> is not nematic in nature and the previously reported diverging elastoresistivity is due to the contamination from the <z:math xmlns:z="http://www.w3.org/1998/Math/MathML" display="inline"><z:msub><z:mi>A</z:mi><z:mrow><z:mn>1</z:mn><z:mi>g</z:mi></z:mrow></z:msub></z:math> channel. Published by the American Physical Society 2024