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Carrier Dynamics and Evaluation of Lasing Actions in Halide Perovskites

Jiajun Qin, Xiaoke Liu, Chunyang Yin, Feng Gao

2020Trends in Chemistry112 citationsDOIOpen Access PDF

Abstract

Metal halide perovskites have shown rapid development in various fields such as photovoltaics, photodetectors, light-emitting diodes (LEDs), and optically pumped lasers owing to their superior optoelectronic properties. Here, we review the basic optoelectronic properties of halide perovskites from a photophysical perspective. We highlight that halide perovskites are promising in various optoelectronic devices functioning at a wide range of carrier densities. We discuss optically and electrically generated carrier density under two different excitation modes [continuous wave (CW) and pulsed] as well as the impact of carrier density on the optoelectronic behavior of perovskites. Moreover, we discuss lasing actions at high carrier densities and summarize key rules to evaluate the lasing actions. Last, we provide an outlook on perovskite-based electrically pumped lasers.

Topics & Concepts

Lasing thresholdOptoelectronicsPerovskite (structure)Materials scienceDiodeLight-emitting diodePhotovoltaicsLaserCarrier lifetimeAuger effectHalideOpticsChemistrySiliconPhysicsPhotovoltaic systemWavelengthCrystallographyEcologyBiologyElectronInorganic chemistryQuantum mechanicsPerovskite Materials and ApplicationsChalcogenide Semiconductor Thin FilmsQuantum Dots Synthesis And Properties
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