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Tandem catalyzing the hydrodeoxygenation of 5-hydroxymethylfurfural over a Ni<sub>3</sub>Fe intermetallic supported Pt single-atom site catalyst

Ge Meng, Kaiyue Ji, Wei Zhang, Yiran Kang, Yu Wang, Ping Zhang, Yang‐Gang Wang, Jun Li, Tingting Cui, Xiaohui Sun, Tianwei Tan, Dingsheng Wang, Yadong Li

2021Chemical Science53 citationsDOIOpen Access PDF

Abstract

A robust Pt<sub>1</sub>/Ni<sub>3</sub>Fe single-atom site catalyst was designed for the tandem catalysis of 5-hydroxymethylfurfural hydrodeoxygenation to DMF, where Pt atoms catalyze the CO group hydrogenation and Ni<sub>3</sub>Fe interface accounts for the C–OH bond rupture.

Topics & Concepts

HydrodeoxygenationCatalysisIntermetallicTandemAtom (system on chip)5-hydroxymethylfurfuralNickelChemistryMaterials scienceOrganic chemistrySelectivityAlloyComputer scienceParallel computingComposite materialCatalysis for Biomass ConversionCatalysis and Hydrodesulfurization StudiesNanomaterials for catalytic reactions
Tandem catalyzing the hydrodeoxygenation of 5-hydroxymethylfurfural over a Ni<sub>3</sub>Fe intermetallic supported Pt single-atom site catalyst | Litcius