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A Sustainable Combustion Process for Green Synthesis of TiO <sub>2</sub> Nanoparticles: Applications in Photocatalytic Degradation and Electrochemical Sensing for Environmental Remediation

Avinash Basavaraja, Chunchanakuppe R. Ravikumar, Afaq Ahmad Khan, Syed Khasim, Bhoomika Vasudeva, Sadanand Sharma, M.S. Santosh

2024ChemistrySelect14 citationsDOI

Abstract

Abstract Herein, a sustainable approach to combustion has been presented, utilizing Aloe Vera latex as a reducing agent in synthesizing titanium dioxide (TiO 2 ) nanoparticles. The phase and composition of TiO 2 have been confirmed using X‐ray diffraction, while the band gap has been determined as 3.17 eV using the Kubelka‐Monk plot. The photocatalytic potential of the TiO 2 has been explored by assessing their effectiveness in degrading AR‐88 dye, demonstrating significant activity at 500 nm. Remarkably, in a span of 120 min of UV radiation, AR‐88 dye could reach an impressive photodegradation rate of 98.6 %, rendering the dye nearly colorless. TiO 2 NPs have also been investigated as an electrode material in sensing paracetamol and D‐glucose by coating them onto a carbon paste electrode and immersing them in a 1 M KOH solution. The cyclic voltammetry experiments reveal that the TiO 2 NPs possess excellent electrochemical characteristics, with a calculated proton diffusion coefficient of 5.651×10 −4 cm 2 s −1 . These findings underscore the potential of TiO 2 as a highly desirable electrode material with remarkable electrochemical properties. This research opens new avenues for utilizing TiO 2 NPs in various electrochemical applications, particularly in the detection of pharmaceutically important compounds, highlighting its versatility.

Topics & Concepts

PhotocatalysisEnvironmental remediationDegradation (telecommunications)NanoparticleElectrochemistryMaterials scienceCombustionProcess (computing)Environmental scienceChemical engineeringNanotechnologyEnvironmental chemistryChemistryContaminationComputer scienceCatalysisEngineeringElectrodeOrganic chemistryBiologyOperating systemPhysical chemistryBiochemistryTelecommunicationsEcologyTiO2 Photocatalysis and Solar CellsNanomaterials for catalytic reactionsAdvanced Photocatalysis Techniques