Recent Advances in Nanomaterial-Based Self-Healing Electrodes Towards Sensing and Energy Storage Applications
Oresegun Olakunle Ibrahim, Chen Liu, Shulan Zhou, Bo Jin, Zhaotao He, Wenjie Zhao, Qianqian Wang, Sheng Zhang
Abstract
Nanomaterial-based self-healing electrodes have demonstrated significant potential in sensing and energy storage applications due to their ability to withstand electrical breakdowns at high electric fields. However, such electrodes often face mechanical challenges, such as cracking under stress, compromising stability and reliability. This review critically examines nanomaterial-based self-healing mechanisms, focusing on properties and applications in health monitoring, motion sensing, environmental monitoring, and energy storage. By comprehensively reviewing research conducted on dimension-based nanomaterials (OD, 1D, 2D, and 3D) for self-healing electrode applications, this paper aims to provide essential insights into design strategies and performance enhancements afforded by nanoscale dimensions. This review paper highlights the tremendous potential of harnessing dimensional nanomaterials to develop autonomously restoring electrodes for next-generation sensing and energy devices.