Litcius/Paper detail

The coil–globule transition in self-avoiding active polymers

S. Das, N. Kennedy, A. Cacciuto

2020Soft Matter34 citationsDOIOpen Access PDF

Abstract

We perform numerical simulations of an active fully flexible self-avoiding polymer as a function of the quality of the embedding solvent described in terms of an effective monomer-monomer interaction. Specifically, by extracting the Flory exponent of the active polymer under different conditions, we are able to pin down the location of the coil-globule transition for different strengths of the active forces. Remarkably, we find that a simple rescaling of the temperature is capable of qualitatively capturing the dependence of the Θ-point of the polymer on the amplitude of active fluctuations. We discuss the limits of this mapping and suggest that a negative active pressure between the monomers, not unlike the one that has already been found in suspensions of active hard spheres, may also be present in active polymers.

Topics & Concepts

PolymerMaterials scienceEmbeddingExponentChemical physicsActive siteSolventQuality (philosophy)AmplitudeFunction (biology)ThermodynamicsCondensed matter physicsStatistical physicsGlass transitionSimple (philosophy)Active learning (machine learning)Optically activePhysicsChemistryTransition temperatureActive matterPolymer chemistryMicro and Nano RoboticsHydrogels: synthesis, properties, applicationsVibration Control and Rheological Fluids