Spin-Orbital Altermagnetism
Zi-Ming Wang, Yang Zhang, Song-Bo Zhang, Jinhua Sun, Elbio Dagotto, Dong-Hui Xu, Lun‐Hui Hu
Abstract
Altermagnetism is a newly discovered magnetic phase, characterized by nonrelativistic spin splitting that has been experimentally observed. Here, we introduce a framework dubbed "spin-orbital altermagnetism" to achieve spin-orbital textures in altermagnetic materials. We identify two distinct classes of spin-orbital altermagnetism: intrinsic and extrinsic. The intrinsic type emerges from symmetry-compensated magnetic orders with spontaneously broken parity-time symmetry, while the extrinsic type stems from translational symmetry breaking between sublattices, as exemplified by the Jahn-Teller-driven structural phase transition. In addition to directly measuring the spin-orbital texture, we propose spin conductivity and spin-resolved orbital polarization as effective methods for detecting these altermagnets. Additionally, a symmetry-breaking mechanism induces weak spin magnetization, further revealing the peculiar feature of spin-orbital altermagnetism. We also utilize the staggered susceptibility to illustrate a potential realization of this phase in a two-orbital interacting system. Our Letter provides a new platform to explore spin-orbital locked physics, extending the materials classes that may display complex spin textures from the standard 4d-5d compounds to 3d compounds.