Litcius/Paper detail

An eco-technoeconomic analysis of hydrogen production using solid oxide electrolysis cells that accounts for long-term degradation

Mina Naeini, James S. Cotton, Thomas A. Adams

2022Frontiers in Energy Research39 citationsDOIOpen Access PDF

Abstract

This paper presents an eco-technoeconomic analysis (eTEA) of hydrogen production via solid oxide electrolysis cells (SOECs) aimed at identifying the economically optimal size and operating trajectories for these cells. Notably, degradation effects were accounted by employing a data-driven degradation-based model previously developed by our group for the analysis of SOECs. This model enabled the identification of the optimal trajectories under which SOECs can be economically operated over extended periods of time, with reduced degradation rate. The findings indicated that the levelized cost of hydrogen (LCOH) produced by SOECs (ranging from 2.78 to 11.67 $/kg H 2 ) is higher compared to gray hydrogen generated via steam methane reforming (SMR) (varying from 1.03 to 2.16 $ per kg H 2 ), which is currently the dominant commercial process for large-scale hydrogen production. Additionally, SOECs generally had lower life cycle CO 2 emissions per kilogram of produced hydrogen (from 1.62 to 3.6 kg CO 2 per kg H 2 ) compared to SMR (10.72–15.86 kg CO 2 per kg H 2 ). However, SOEC life cycle CO 2 emissions are highly dependent on the CO 2 emissions produced by its power source, as SOECs powered by high-CO 2 -emission sources can produce as much as 32.22 kg CO 2 per kg H 2 . Finally, the findings of a sensitivity analysis indicated that the price of electricity has a greater influence on the LCOH than the capital cost.

Topics & Concepts

Hydrogen productionHydrogenElectrolysisChemistryEnvironmental scienceMaterials scienceElectrodeElectrolyteOrganic chemistryPhysical chemistryAdvancements in Solid Oxide Fuel CellsChemical Looping and Thermochemical ProcessesCO2 Reduction Techniques and Catalysts