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Highly Efficient Aggregation-Induced Red-Emissive Organic Thermally Activated Delayed Fluorescence Materials with Prolonged Fluorescence Lifetime for Time-Resolved Luminescence Bioimaging

Sujie Qi, Sangin Kim, Nguyễn Văn Nghĩa, Youngmee Kim, Guangle Niu, Gyoungmi Kim, Sung‐Jin Kim, Sungnam Park, Juyoung Yoon

2020ACS Applied Materials & Interfaces109 citationsDOI

Abstract

to promote the occurrence of reverse intersystem crossing (RISC). Moreover, they all exhibit aggregation-induced red emissions and long delayed fluorescence lifetimes without the influence of molecular oxygen. More importantly, these long-lived and biocompatible TADF materials, especially the phenoxazine-substituted NI fluorophores, show great potential for high-contrast fluorescence lifetime imaging in living cells. This study provides further a molecular design strategy for purely organic TADF materials and expands the versatile biological application of long-lived fluorescence research in time-resolved luminescence imaging.

Topics & Concepts

PhenoxazineFluorescenceIntersystem crossingMaterials scienceLuminescencePhotochemistryBiological imagingAcceptorFluorescence-lifetime imaging microscopyOLEDPhenothiazineNanotechnologyOptoelectronicsChemistryOpticsLayer (electronics)PharmacologySinglet stateExcited stateCondensed matter physicsMedicineNuclear physicsPhysicsLuminescence and Fluorescent MaterialsOrganic Light-Emitting Diodes ResearchMolecular Sensors and Ion Detection
Highly Efficient Aggregation-Induced Red-Emissive Organic Thermally Activated Delayed Fluorescence Materials with Prolonged Fluorescence Lifetime for Time-Resolved Luminescence Bioimaging | Litcius