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Divergent Synthesis of Trifluoromethyl-Substituted 1,2-Dihydroquinoxalines and Diimines by Cascade Reactions of CF<sub>3</sub>–Imidoyl Sulfoxonium Ylides with Azo Compounds

Guangming Wei, Dongling Zheng, Chen Li, Zhengkai Chen, Xiao‐Feng Wu

2023Organic Letters20 citationsDOI

Abstract

-imidoyl sulfoxonium ylides and azo compounds has been achieved, allowing for facile access to trifluoromethyl-substituted 1,2-dihydroquinoxalines and diimines in moderate to excellent yields. Noteworthy is that the unusual N-N bond cleavage and rearrangement of azo compounds are involved in the transformations.

Topics & Concepts

ChemistryTrifluoromethylCascadeCleavage (geology)Bond cleavageCombinatorial chemistryMedicinal chemistryBase (topology)StereochemistryOrganic chemistryCatalysisMathematicsMathematical analysisFracture (geology)AlkylChromatographyGeotechnical engineeringEngineeringFluorine in Organic ChemistryCyclopropane Reaction MechanismsSynthesis and Biological Evaluation
Divergent Synthesis of Trifluoromethyl-Substituted 1,2-Dihydroquinoxalines and Diimines by Cascade Reactions of CF<sub>3</sub>–Imidoyl Sulfoxonium Ylides with Azo Compounds | Litcius