Litcius/Paper detail

Thin‐Film Thermoelectric Generators Comprising Molybdenum‐Based MXenes pn Modules

park taeho, Kyoungah Cho, Sangsig Kim

2021Advanced Materials Technologies24 citationsDOI

Abstract

Abstract In this study, the thermoelectric characteristics of spin‐coated p‐Mo 2 C and n‐Mo 2 Ti 2 C 3 thin films and the scalability of MXene thin‐film thermoelectric generators (TFTEGs) constructed with pn modules are investigated. The in‐plane thermal conductivities are measured at room temperature to be 0.37 and 0.45 W (m K) −1 for the p‐Mo 2 C and n‐Mo 2 Ti 2 C 3 thin films, respectively. The dimensionless figures of merit ZT are determined to be 1.7 × 10 −5 and 2.6 × 10 −4 for the p‐Mo 2 C and n‐Mo 2 Ti 2 C 3 thin films, respectively. The scalability of the MXene TFTEG is evaluated by the Seebeck voltage being directly proportional to the number of pn modules. The MXene TFTEG constructed with 200‐pn modules generates a Seebeck voltage of 399.9 mV and an output power of 6 mW cm −2 at a Δ T of 5.4 K.

Topics & Concepts

Thermoelectric effectMaterials scienceThin filmMolybdenumThermoelectric generatorSeebeck coefficientMXenesThermoelectric materialsOptoelectronicsAnalytical Chemistry (journal)Thermal conductivityNanotechnologyMetallurgyComposite materialChemistryThermodynamicsPhysicsChromatographyMXene and MAX Phase Materials2D Materials and ApplicationsAdvanced Thermoelectric Materials and Devices