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Simultaneously Enhancing Brightness and Purity of WSe<sub>2</sub> Single Photon Emitter Using High-Aspect-Ratio Nanopillar Array on Metal

Mayank Chhaperwal, Himanshu Madhukar Tongale, Patrick Hays, Kenji Watanabe, Takashi Taniguchi, Sefaattin Tongay, Kausik Majumdar

2024Nano Letters11 citationsDOI

Abstract

A monolayer semiconductor transferred on nanopillar arrays provides site-controlled, on-chip single photon emission, which is a scalable light source platform for quantum technologies. However, the brightness of these emitters reported to date often falls short of the perceived requirement for such applications. Also, the single photon purity usually degrades as the brightness increases. Hence, there is a need for a design methodology to achieve an enhanced emission rate while maintaining high single photon purity. By using WSe 2 on high-aspect-ratio (∼3, at least 2-fold higher than previous reports) nanopillar arrays, here we demonstrate >10 MHz single photon emission rate in the 770–800 nm band that is compatible with quantum memory and repeater networks (Rb-87-D1/D2 lines) and satellite quantum communication. The emitters exhibit excellent purity (even at high emission rates) and improved out-coupling due to the use of a gold back reflector that quenches the emission away from the nanopillar.

Topics & Concepts

NanopillarCommon emitterBrightnessMaterials scienceAspect ratio (aeronautics)MetalPhotonOpticsOptoelectronicsNanotechnologyAnalytical Chemistry (journal)PhysicsNanostructureChemistryChromatographyMetallurgy2D Materials and ApplicationsNanowire Synthesis and ApplicationsChalcogenide Semiconductor Thin Films
Simultaneously Enhancing Brightness and Purity of WSe<sub>2</sub> Single Photon Emitter Using High-Aspect-Ratio Nanopillar Array on Metal | Litcius