Litcius/Paper detail

Superwetting Patterned Membranes with an Anisotropy/Isotropy Transition: Towards Signal Expression and Liquid Permeation

Ruixiang Qu, Xiangyu Li, Yanan Liu, Huajun Zhai, Shuaiheng Zhao, Lin Feng, Yen Wei

2020Angewandte Chemie International Edition32 citationsDOI

Abstract

Abstract Superwetting membranes with responsive properties have attracted heightened attention because of their fine‐tunable surface wettability. However, their functional diversity is severely limited by the “black‐or‐white” wettability transition. Herein, we describe a coating strategy to fabricate multifunctional responsive superwetting membranes with SiO 2 /octadecylamine patterns. The adjustable patterns in the responsive region are the key factor for functional diversity. Specifically, the coated part of the membrane displayed a superhydrophobicity/superhydrophilicity transition at different pH values, whereas the uncoated part exhibited invariant superhydrophilicity. On the basis of this anisotropy/isotropy transition, the membranes can serve as either responsive permeable membranes or signal‐expression membranes, thus enabling the responsive separation and permeation of liquids with satisfactory separation efficiency (>99.90 %) and flux (ca. 60 L m −2 h), as well as real‐time liquid signal expression with alterable signals.

Topics & Concepts

MembraneSuperhydrophilicityWettingIsotropyPermeationMaterials scienceAnisotropyChemical engineeringBiophysicsChemistryNanotechnologyChromatographyOpticsComposite materialBiochemistryPhysicsEngineeringBiologySurface Modification and SuperhydrophobicityMembrane Separation TechnologiesAdvanced Sensor and Energy Harvesting Materials