Litcius/Paper detail

In Situ Transmission Electron Microscopy for Ultrahigh Temperature Mechanical Testing of ZrO<sub>2</sub>

Robson L. Grosso, E.N.S. Muccillo, Dereck N.F. Muche, Gowtham S. Jawaharram, Christopher M. Barr, Anthony M. Monterrosa, Ricardo H. R. Castro, Khalid Hattar, Shen J. Dillon

2020Nano Letters29 citationsDOIOpen Access PDF

Abstract

This work demonstrates a novel approach to ultrahigh-temperature mechanical testing using a combination of in situ nanomechanical testing and localized laser heating. The methodology is applied to characterizing and testing initially nanograined 10 mol % Sc2O3-stabilized ZrO2 up to its melting temperature. The results suggest that the low-temperature strength of nanograined, d < 50 nm, oxides is not influenced by creep. Tensile fracture of ZrO2 bicrystals produce a weak-temperature dependence suggesting that grain boundary energy dominates brittle fracture of grain boundaries even at high homologous temperatures; for example, T = 2050 °C or T ≈ 77% Tmelt. The maximum temperature for mechanical testing in this work is primarily limited by the instability of the sample, due to evaporation or melting, enabling a host of new opportunities for testing materials in the ultrahigh-temperature regime.

Topics & Concepts

Materials scienceGrain boundaryBrittlenessTensile testingCreepWork (physics)Transmission electron microscopyGrain Boundary SlidingUltimate tensile strengthComposite materialMicrostructureNanotechnologyThermodynamicsPhysicsAdvanced ceramic materials synthesisNuclear Materials and PropertiesHigh-Temperature Coating Behaviors