Litcius/Paper detail

Large Spin‐to‐Charge Conversion at Room Temperature in Extended Epitaxial Sb<sub>2</sub>Te<sub>3</sub> Topological Insulator Chemically Grown on Silicon

Emanuele Longo, Matteo Belli, Mario Alia, Martino Rimoldi, Raimondo Cecchini, Massimo Longo, Claudia Wiemer, Lorenzo Locatelli, Polychronis Tsipas, A. Dimoulas, G. Gubbiotti, M. Fanciulli, R. Mantovan

2021Advanced Functional Materials41 citationsDOIOpen Access PDF

Abstract

Abstract Spin‐charge interconversion phenomena at the interface between magnetic materials and topological insulators (TIs) are attracting enormous interest in the research effort toward the development of fast and ultra‐low power devices for future information and communication technology. A large spin‐to‐charge (S2C) conversion efficiency in Au/Co/Au/Sb 2 Te 3 /Si(111) heterostructures based on Sb 2 Te 3 TIs grown by metal–organic chemical vapor deposition on 4″ Si(111) substrates is reported. By conducting room temperature spin pumping ferromagnetic resonance, a 250% enhanced charge current due to spin pumping in the Sb 2 Te 3 ‐containing system is measured when compared to the reference Au/Co/Au/Si(111). The corresponding inverse Edelstein effect length λ IEE ranges from 0.28 to 0.61 nm, depending on the adopted methodological analysis, with the upper value being so far the largest observed for the second generation of 3D chalcogenide‐based TIs. These results open the path toward the use of chemical methods to produce TIs on large area Si substrates and characterized by highly performing S2C conversion, thus marking a milestone toward future technology‐transfer.

Topics & Concepts

Topological insulatorChemical vapor depositionChalcogenideEpitaxyHeterojunctionSpin pumpingMaterials scienceOptoelectronicsSiliconCondensed matter physicsAnalytical Chemistry (journal)NanotechnologySpin Hall effectChemistrySpin polarizationElectronPhysicsQuantum mechanicsLayer (electronics)ChromatographyTopological Materials and PhenomenaAdvanced Condensed Matter PhysicsMagnetic properties of thin films
Large Spin‐to‐Charge Conversion at Room Temperature in Extended Epitaxial Sb<sub>2</sub>Te<sub>3</sub> Topological Insulator Chemically Grown on Silicon | Litcius