Litcius/Paper detail

Photoswitchable phosphines in catalysis

Fabrizio Medici, Nawel Goual, Vincent Delattre, Arnaud Voituriez, Angéla Marinetti

2020ChemCatChem30 citationsDOIOpen Access PDF

Abstract

Abstract Photoswitchable catalysts based on phosphorus ligands have been overlooked so far, despite the growing current interest for catalysts control through external stimuli. This review surveys the current knowledge in the field, including synthetic approaches to photoswitchable phosphines and their transition metal complexes, and applications in rhodium, palladium, gold, ruthenium and copper catalysis. This survey demonstrates that both regulation of the catalytic activity and tuning of the chemo‐ and enantioselectivity can be achieved using irradiation as a non‐invasive external stimulus. Non‐catalytic uses of photoswitchable phosphines in organic synthesis are also mentioned.

Topics & Concepts

CatalysisRhodiumRutheniumChemistryPalladiumTransition metalCombinatorial chemistryNanotechnologyOrganic chemistryMaterials sciencePhotochromic and Fluorescence ChemistryPhotoreceptor and optogenetics researchMolecular Sensors and Ion Detection