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Theoretical insights into the structural, optoelectronic, thermoelectric, and thermodynamic behavior of novel quaternary LiZrCoX (X = Ge, Sn) compounds based on first-principles study

Meena Kumari, Jisha Annie Abraham, Ramesh Sharma, Debidatta Behera, Sanat Kumar Mukherjee, Mostafa M. Salah, Murefah mana Al‐Anazy, Mohammed S. Alqahtani

2023RSC Advances30 citationsDOIOpen Access PDF

Abstract

) and the linked elastic moduli show their stability in the cubic phase. The calculated value of Pugh's ratio and Cauchy pressure reveal that LiZrCoGe is brittle whereas LiZrCoSn is ductile. Additionally, the optical characteristics of the compounds are studied in terms of the dielectric function, refractive index, extinction coefficient, absorption coefficient, reflectivity, energy loss function, and optical conductivity. The obtained high value of power factor and figure of merit of the studied lithium-based quaternary compounds predict good thermoelectric behavior in these compounds. Thus, LiZrCoX (X = Ge, Sn) compounds can therefore be used to create innovative and intriguing thermoelectric materials as well as optoelectronic and energy-harvesting equipment.

Topics & Concepts

Thermoelectric effectMaterials scienceQuaternaryOptoelectronicsNanotechnologyThermodynamicsPhysicsGeologyPaleontologyHeusler alloys: electronic and magnetic propertiesChalcogenide Semiconductor Thin FilmsSemiconductor materials and interfaces
Theoretical insights into the structural, optoelectronic, thermoelectric, and thermodynamic behavior of novel quaternary LiZrCoX (X = Ge, Sn) compounds based on first-principles study | Litcius