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Dual NHC/photoredox catalytic synthesis of 1,4-diketones using an MR-TADF photocatalyst (DiKTa)

Callum Prentice, J. A. Morrison, Eli Zysman‐Colman, Andrew D. Smith

2022Chemical Communications25 citationsDOIOpen Access PDF

Abstract

The use of the recently reported organic multi-resonant thermally activated delayed fluorescent (MR-TADF) photocatalyst DiKTa allows for the modular synthesis of 1,4-diketones under mild and metal-free conditions.

Topics & Concepts

CatalysisPhotocatalysisChemistryCarbenePhotochemistryFluorescenceComponent (thermodynamics)Combinatorial chemistryModular designOrganic chemistryOperating systemPhysicsThermodynamicsComputer scienceQuantum mechanicsCatalytic C–H Functionalization MethodsRadical Photochemical ReactionsSulfur-Based Synthesis Techniques