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Responsive photoactive probe based photoelectrochemical sensor for sulfur dioxide

Yingying Zhang, Yuanqiang Hao, Ying Peng, Xiaobing Wang, Yanli Zhou, Shu Chen, Maotian Xu

2024Electroanalysis13 citationsDOIOpen Access PDF

Abstract

Abstract This study introduces a novel photoelectrochemical (PEC) sensor for the highly selective detection of sulfur dioxide (SO 2 ) using an organic photoactive molecule probe (OPM). OPM is synthesized through a one‐step coupling reaction, featuring a typical photosensitizer D‐π‐A structure. By covalently bonding OPM with a TiO 2 substrate, a PEC sensor is constructed, exhibiting a significant photocurrent response under visible light excitation. The specific addition reaction between SO 2 and OPM disrupts its conjugated structure, reducing the photocurrent response and achieving highly selective detection of SO 2 . The sensor demonstrates excellent performance in real water samples, emphasizing its practical applications.

Topics & Concepts

PhotocurrentSulfur dioxideMoleculePhotosensitizerMaterials sciencePhotochemistryChemistrySubstrate (aquarium)PhotoelectrochemistryCovalent bondElectrochemistryOptoelectronicsInorganic chemistryElectrodeOrganic chemistryPhysical chemistryOceanographyGeologyPerovskite Materials and ApplicationsOrganic Chemistry Cycloaddition ReactionsAnalytical Chemistry and Sensors
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