Litcius/Paper detail

Testing the isomorph invariance of the bridge functions of Yukawa one-component plasmas

Federico Lucco Castello, P. Tolias, Jeppe C. Dyre

2021The Journal of Chemical Physics23 citationsDOIOpen Access PDF

Abstract

It has been recently conjectured that bridge functions remain nearly invariant along phase diagram lines of constant excess entropy for the broad class of R-simple liquids. To test this hypothesis, the bridge functions of Yukawa systems are computed outside the correlation void with the Ornstein-Zernike inversion method employing structural input from ultra-accurate molecular dynamics simulations and inside the correlation void with the cavity distribution method employing structural input from ultra-long specially designed molecular dynamics simulations featuring a tagged particle pair. Yukawa bridge functions are revealed to be isomorph invariant to a very high degree. The observed invariance is not exact, however, since isomorphic deviations exceed the overall uncertainties.

Topics & Concepts

Yukawa potentialComponent (thermodynamics)Bridge (graph theory)PlasmaPhysicsParticle physicsMathematicsQuantum mechanicsBiologyAnatomyDust and Plasma Wave PhenomenaVacuum and Plasma ArcsHigh-pressure geophysics and materials