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Observation of Strong Valley Magnetic Response in Monolayer Transition Metal Dichalcogenide Alloys of Mo<sub>0.5</sub>W<sub>0.5</sub>Se<sub>2</sub> and Mo<sub>0.5</sub>W<sub>0.5</sub>Se<sub>2</sub>/WS<sub>2</sub> Heterostructures

Lishu Wu, Chunxiao Cong, Weihuang Yang, Yu Chen, Yan Shao, T. Thu Ha, Wen Wen, Shun Feng, Chenji Zou, Hongbo Zhang, Bowen Du, Bingchen Cao, Jingzhi Shang, Qihua Xiong, Kian Ping Loh, Ting Yu

2021ACS Nano18 citationsDOI

Abstract

. Such interlayer charge transfer further evidences the formation of type-II band alignment, in agreement with the density functional theory calculations. Our findings give insights into the spin-valley and interlayer coupling effects in monolayer TMD alloys and their heterostructures, which are essential to develop valleytronic applications based on the emerging family of TMD alloys.

Topics & Concepts

MonolayerTrionZeeman effectHeterojunctionCondensed matter physicsSpintronicsMaterials scienceExcitonDensity functional theoryTransition metalFerromagnetismMagnetic fieldChemistryNanotechnologyPhysicsComputational chemistryBiochemistryCatalysisQuantum mechanics2D Materials and ApplicationsPerovskite Materials and ApplicationsMXene and MAX Phase Materials
Observation of Strong Valley Magnetic Response in Monolayer Transition Metal Dichalcogenide Alloys of Mo<sub>0.5</sub>W<sub>0.5</sub>Se<sub>2</sub> and Mo<sub>0.5</sub>W<sub>0.5</sub>Se<sub>2</sub>/WS<sub>2</sub> Heterostructures | Litcius