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Rational design of a photoswitchable DNA glue enabling high regulatory function and supramolecular chirality transfer

Nadja A. Simeth, Shotaro Kobayashi, Piermichele Kobauri, Stefano Crespi, Wiktor Szymański, Kazuhiko Nakatani, Chikara Dohno, Ben L. Feringa

2021Chemical Science29 citationsDOIOpen Access PDF

Abstract

We present the rational design of photoswitchable DNA glue to trigger the reversible formation of duplex DNA by light. The supramolecular assembly shows a mutual interaction between ligand and DNA, which induces a preferred helicity in the switch.

Topics & Concepts

Rational designSupramolecular chemistryDNADuplex (building)Chirality (physics)ChemistrySupramolecular chiralityHelix (gastropod)Molecular machineNanotechnologyBiophysicsMaterials scienceCrystallographyBiologyPhysicsBiochemistryEcologySnailQuantum mechanicsChiral symmetry breakingNambu–Jona-Lasinio modelQuarkCrystal structurePhotochromic and Fluorescence ChemistryPhotoreceptor and optogenetics researchDNA and Nucleic Acid Chemistry
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